Metals in nature exhibit a mediocre wettability and a high optical reflectance from the visible region to the infrared. This Letter reports that, by formation of nano- and microscale structures via a simple raster scanning of a focused femtosecond laser pulse without any further treatment, structured aluminum and nickel surfaces exhibit combined features of superhydrophobicity with a contact angle of 155.5°, and a high optical absorption with a reflectivity of several percent over a broad spectral range (0.2–2.5 μm). Thus, a multifunctional structured metal surface that integrates superhydrophobicity and a high broadband absorptivity has been easily realized by one-step femtosecond laser processing.